This study employed the Taguchi method to determine the optimal milling parameters for cast steel, aiming to minimize surface roughness. The analysis indicated that the feed rate was the most significant factor, with lower feed rates resulting in improved surface finish. In contrast, spindle speed and radial depth of cut had minimal impact, while axial depth of cut and tempering temperature emerged as crucial determinants. A linear regression model accounted for 87.46% of the variance in surface roughness. The predicted optimal conditions closely aligned with experimental results, yielding only a 2.93% error and achieving an average surface roughness of 3.033 μm. These findings provide a predictive framework for achieving the desired surface quality in milling processes.