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A Review of in Operando Measurements of Local Temperature for Lithium-ion Batteries
Soyoung Park, Woosung Park
J. Korean Soc. Precis. Eng. 2025;42(12):1021-1035.
Published online December 1, 2025
DOI: https://doi.org/10.7736/JKSPE.025.00024
Sensing the internal temperature of lithium-ion batteries is particularly useful for reliable battery operation as both electrochemistry and mass transport are dictated by local temperature. In this article, we review in operando techniques to monitor the internal temperature of lithium-ion batteries during charging and discharging. We categorize existing techniques into two groups: invasive and non-invasive approaches. Invasive techniques include optical fibers, thermocouples, and resistance temperature detectors as a thermometer. Non-invasive methods cover the temperature estimation techniques, namely electrochemical impedance spectroscopy as well as X-ray thermometry. For both approaches, we review working principle of thermometry, pros and cons of each thermometry, and recent studies to tackle relevant technical challenges. This review provides useful information for internal temperature measurements, offering chances for thermally reliable battery operation.
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Dendrite Growth Suppression in Lithium Metal Batteries with Composite Quasi-solid Electrolytes
Jeongeun Park, Jinhyeong An, Jiwoong Bae
J. Korean Soc. Precis. Eng. 2025;42(12):1037-1043.
Published online December 1, 2025
DOI: https://doi.org/10.7736/JKSPE.025.00010
Secondary batteries are crucial for eco-friendly systems, but existing technologies struggle with energy density and safety issues. This study aims to develop a next-generation battery utilizing quasi-solid electrolytes (QSE), which combine the advantages of both liquid and solid electrolytes. However, QSEs often lack the mechanical strength necessary to prevent lithium dendrite growth. To address this challenge, two strategies were proposed and experimentally validated. The first strategy involves creating a QSE-separator composite (QSE-PI) by integrating QSE with a polyimide (PI) separator. Among the various options, PI with a thickness greater than 20 μm and a pore size of 2-5 μm exhibited superior electrolyte absorption and dendrite suppression. This configuration allowed for rapid lithium plating/stripping, high ionic conductivity (1.7 × 10-3 S cm-1), and excellent Coulombic efficiency (99.94%).The second strategy incorporates silica (SiO2) as a ceramic filler in the QSE-PI to enhance mechanical strength and ion transport. The addition of SiO2 disrupted polymer crystallinity, increased the amorphous regions, and effectively suppressed dendrite formation. Notably, SiO2 particles larger than 10 μm improved cycle stability, with the composite maintaining performance for over 50 cycles, compared to only 30 cycles for the version without filler.
  • 168 View
  • 15 Download

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Suppression of Interfacial Side Reactions and Performance Enhancement of NCA Cathodes via LNO Deposition Using Particle ALD
Min-ji Kim, In-suk Song, Hyo-jun Ahn, Sun-min Kim, Young-Beom Kim
J. Korean Soc. Precis. Eng. 2025;42(10):851-859.
Published online October 1, 2025
DOI: https://doi.org/10.7736/JKSPE.025.025

Improving the interfacial stability between cathode active material (CAM) and solid electrolyte (SE) is essential for enhancing the performance and durability of all-solid-state batteries (ASSBs). One promising method to achieve this is through surface coating with a chemically stable ion conductor, which helps suppress interfacial side reactions and improve long-term cycling stability. In this study, we deposited a uniform LiNbO3 (LNO) protective layer on NCA using particle atomic layer deposition (Particle ALD). This technique utilizes a self-limiting growth mechanism to ensure precise thickness control. We characterized the structural and chemical properties of the coated CAM with X-ray photoelectron spectroscopy (XPS), X-ray diffraction (XRD), and scanning electron microscopy-energy dispersive spectroscopy (SEM-EDS), confirming the successful formation of a uniform LNO layer. Electrochemical evaluations revealed that LNO@NCA exhibited significantly improved capacity retention, maintaining 68.1% after 50 cycles at a 1C rate, compared to just 56.5% for the uncoated sample. This enhancement is attributed to the LNO layer's effectiveness in mitigating electrochemical side reactions. These findings demonstrate that Particle ALD-derived LNO coatings are an effective strategy for stabilizing CAM|SE interfaces and extending the cycle life of high-energy ASSBs.

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Power Consumption Analysis and Optimal Operation Method of Wireless Multi-sensor Module
Hyun Sik Son, Duck-Keun Kim, Kwang Eun Ko, Seung-Hwan Yang
J. Korean Soc. Precis. Eng. 2025;42(10):843-849.
Published online October 1, 2025
DOI: https://doi.org/10.7736/JKSPE.025.023

Smart farms and smart factories utilize various environmental measurement and task recognition sensors. For situations requiring simultaneous measurements, a multi-sensor module that combines several sensors into one unit is advantageous. This study focuses on integrating various sensors into a single module and proposing an optimal usage method to minimize the power consumption of a wireless multi-sensor module capable of remote measurements. Analysis of the power consumption of individual sensor components revealed that when the measurement interval exceeds one minute, power consumption can be reduced by over 50.3% by turning off sensors during idle periods. If real-time responsiveness is not essential, the most efficient approach is to keep the entire module in sleep mode during these idle periods. A practical experiment was conducted using a multi-sensor module equipped with temperature and humidity, illuminance, CO2 concentration, and soil moisture sensors. When continuously powered, the module operated for 40 hours on a 3500 mAh Li-ion battery. However, by implementing sleep mode with a five-minute measurement interval, the operational duration extended to 562 hours.

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Thermal Runaway Characteristics Induced by Heat Abuse Conditions in 18650 Li-ion Batteries
Jungmyung Kim, Heesung Park
J. Korean Soc. Precis. Eng. 2023;40(10):821-827.
Published online October 1, 2023
DOI: https://doi.org/10.7736/JKSPE.022.145
This study aimed to characterize the mechanism of thermal runaway phenomenon in lithium-ion batteries, which represent secondary cells among energy storage devices. Thermal runaway reaction was induced by heating 18650 cells with 5%, 40%, and 80% state of charge (SOC). We divided the thermal runaway of the battery into three stages and discussed the physical measurements that distinguish each stage. We also provided a visual comparison and thermal image of the characterized exhaust gases in all stages. The state of charge and the amount of heat generated by thermal runaway were proportional, and in the third stage of thermal runaway, where the highest mass transfer occurred, 40% of SOC released gas for 13 seconds and 80% of SOC emitted gas and flame for 3 seconds. In addition, a temperature and voltage measurement method that can predict the thermal runaway phenomenon of a battery is presented.

Citations

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  • An Experimental Study on the Thermal Runaway Characteristics of Single and Multiple Lithium-Ion Cells
    Ho-Sik Han, Gyu-Hwan Cho, Hong-Seok Yun
    Fire Science and Engineering.2025; 39(5): 13.     CrossRef
  • Quantitative Evaluation of Vent-to-Thermal Runaway Transition and the Delay/Suppression Effects of Cooling Extinguishing Agents in Forced-Heated 18650 Cells
    TaeYuun Ham, Jong-Hyo Choi, DoHyun Kim, ChanSol Ahn
    Journal of the Korean Society of Hazard Mitigation.2025; 25(6): 199.     CrossRef
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A Study on the Selection of Failure Factors for Transient State Lithium-Ion Batteries based on Electrochemical Impedance Spectroscopy
Miyoung Lee, Seungyun Han, Jinhyeong Park, Jonghoon Kim
J. Korean Soc. Precis. Eng. 2021;38(10):749-756.
Published online October 1, 2021
DOI: https://doi.org/10.7736/JKSPE.021.040
Lithium-ion batteries are one of the main parts of electrical devices and are widely used in various applications. To safely use lithium-ion batteries, fault diagnosis and prognosis are significant. This paper analyzes resistance parameters from electrochemical impedance spectroscopy (EIS) to detect the fault of lithium-ion batteries. The internal fault mechanisms of batteries are so complex; it is difficult to detect abnormalities by direct current-based methods. However, by using alternating-current-based impedance by EIS, the internal degradation processes of the batteries can be detected. Impedance variation from EIS is verified under accelerated degradation test conditions and normal cycling test conditions. The results showed a significant relationship between fault and increase in resistance.

Citations

Citations to this article as recorded by  Crossref logo
  • Research into the Detection of Faulty Cells in Battery Systems Using BMS Cell Balancing Counts
    Hyunjun Kim, Woongchul Choi
    Transaction of the Korean Society of Automotive Engineers.2025; 33(8): 637.     CrossRef
  • PEDOT:PSS‐Based Prolonged Long‐Term Decay Synaptic OECT with Proton‐Permeable Material, Nafion
    Ye Ji Lee, Yong Hyun Kim, Eun Kwang Lee
    Macromolecular Rapid Communications.2024;[Epub]     CrossRef
  • Lithium-Ion Batteries (LIBs) Immersed in Fire Prevention Material for Fire Safety and Heat Management
    Junho Bae, Yunseok Choi, Youngsik Kim
    Energies.2024; 17(10): 2418.     CrossRef
  • 90 View
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Damage-Free Freeform Cutting of Flexible Battery Using Ultra-Short Pulse Laser
SeokYoung Ji, Jaegu Kim, Sung Hak Cho, Hyungjun Lim, Won Seok Chang
J. Korean Soc. Precis. Eng. 2021;38(3):195-202.
Published online March 1, 2021
DOI: https://doi.org/10.7736/JKSPE.020.099
With the progress of flexible devices, numerous researchers aim to manufacture the flexible battery with freefrom at various scales. Laser cutting is considered as one of the essential processes to achieve on-demand manufacturing but continuous wave or long-pulse laser beam may cause large heat affect zone (HAZ) in cutting edge and may even result in failure of battery function. Herein, it was demonstrated that the sophisticated cutting process using ultra-short pulse laser is applicable for tailoring of flexible battery with multilayered structure. Based on the comparison of cutting results using nanosecond laser and femtosecond laser, we confirmed that laser cutting by femtosecond laser induces much less thermal damage on thin foil electrodes, separator, and electrolyte. Furthermore, we investigated the interaction of femtosecond laser with the materials composed of a flexible battery and implemented a process for cutting each material without causing any critical damage. To prevent a short circuit between the anode and cathode, which usually occurs during laser cutting of the actual battery, the double-side cutting process was done by adjusting the focal points of the laser beam. We assume that the proposed approach can be applied in a roll-to-roll based cutting process for the mass-production of flexible devices.
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The Effect of Thickness of Electrodes on Edge Quality in Laser Cutting of Electrodes
Dongkyu Park, Dongkyoung Lee
J. Korean Soc. Precis. Eng. 2021;38(2):97-101.
Published online February 1, 2021
DOI: https://doi.org/10.7736/JKSPE.020.095
Many countries are trying to overcome global warming due to greenhouse gas emissions, such as CO₂. In particular, the regulation on CO₂ emissions of internal combustion engine vehicles has become strictly important. Thus, the automobile companies are putting more effort for improving the manufacturing of the battery, which is the main power supply of electrical vehicles. In the electrode cutting process, laser cutting has been actively discussed to solve problems originating from the conventional electrode cutting processes. However, there is a lack of research considering the effect of thickness of the active material on laser cutting. In this paper, the effect of thickness of the active material on laser cutting of electrodes is analyzed. First, the cut electrodes are observed through a scanning electron microscope (SEM). Next, the kerf width and clearance width of the electrodes are measured and compared at the same laser parameter. The kerf width and clearance width of relatively thick electrodes are narrowly formed. Finally, the cutting quality of the electrode is compared. A uniform cut edge is observed as the scanning speed increases.

Citations

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  • Comparison of laser processability for LiFePO4 cathode material with nanosecond and femtosecond laser
    Jaegeun Shin, Juhee Yang, Dongkyoung Lee
    Journal of Science: Advanced Materials and Devices.2024; 9(3): 100753.     CrossRef
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Optimization Design for Augmentation of Cooling Performance Utilizing Leading-Edge Materials in Electric Vehicle Battery Cells
Byeong Yeop Kim, Dong-Ryul Lee
J. Korean Soc. Precis. Eng. 2020;37(7):529-538.
Published online July 1, 2020
DOI: https://doi.org/10.7736/JKSPE.020.044
This study is to investigate the cooling performance of the battery in the electric vehicle depending on the attachment of the cooling plates and materials to the battery cells. Research focused on the numerical comparison of forced convective heat transfer coefficients with case 1(cell-Al, cooling plate-None), case 2(cell-Al, cooling plate-Al), case 3(cell-Al, cooling plate-C), and case 4(cell-C, cooling plate-Al). Normalized local Nusselt number of the cooling area at the normalized width position indicated that the heat transfer coefficient of the case 1 was averaging at 7, 14.5, 11.9% lower than that of case 2, case 3, and case 4. Based on case 3, the cooling performance with six different types of mass flow rates (0.05, 0.075, 0.0875, 0.1, 0.125, 0.15 kg/s) were compared. Normalized local Nusselt number at the normalized width position indicated that the heat transfer coefficient of 0.0875 kg/s was averaging at 35.8, 11.9% higher than that of 0.05, 0.075 kg/s and 12.3, 36.4, 60% lower than that of 0.1, 0.125, 0.15 kg/s. Ultimately, the best optimization design for air-cooling performance was case 3 with mass flow rate of 0.125 kg/s.

Citations

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  • Numerical and Experimental Approaches for Mechanical Durability Assessment of an EV Battery Pack Case
    Hyun Soo Kim, Mingoo Cho, Changyeon Lee, Jaewoong Kim, Sungwook Kang
    Materials.2025; 18(24): 5683.     CrossRef
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A Study on Heat Radiation Performance for Different Layout of Electric Vehicle Secondary Battery Cell
Seung Bong Hyun, Byeong Yeop Kim, Ji Hun Song, Dong-Ryul Lee
J. Korean Soc. Precis. Eng. 2020;37(4):271-282.
Published online April 1, 2020
DOI: https://doi.org/10.7736/JKSPE.020.007
This study is to investigate the cooling performance of the secondary battery in electric vehicles according to three different gaps between battery cells. To accomplish the convective cooling performance of the battery surface with three different gaps, selected local positions (X, Y, Z) for various temperature distributions were marked on the gap surface contacting the cell surface. The cooling performance of the gap of 0.5 mm was compared with the gaps of 5 mm, and 1 mm. Normalized local Nusselt number of the cooling area at the normalized width position indicated that the gap of 0.5 mm was on average 26.99% lower than that of 5 mm and 0.49% lower than that of 1 mm. At the normalized height, the gap of 0.5 mm was on average 12.12% higher than that of 1 mm. Because of the vortex at the outlet area, cooling performance at the gap of 0.5 mm was on average 13.19% higher than that of 5 mm and 0.79% higher than that of 1 mm at normalized thickness. Ultimately, the best cooling performance existed at the gap of 5 mm, but the gap of 0.5 mm was best for improving space efficiency, energy storage capacity, and vehicle-driving durability.

Citations

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  • A Study on Cooling Performance Augmentation of Water-Cooling and Optimization Design Utilizing Carbon Material in Electric Vehicle Secondary Battery
    Seung Bong Hyun, Dong-Ryul Lee
    Journal of the Korean Society for Precision Engineering.2020; 37(7): 519.     CrossRef
  • Optimization Design for Augmentation of Cooling Performance Utilizing Leading-Edge Materials in Electric Vehicle Battery Cells
    Byeong Yeop Kim, Dong-Ryul Lee
    Journal of the Korean Society for Precision Engineering.2020; 37(7): 529.     CrossRef
  • 66 View
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